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The 27th AIRAPT International Conference on High Pressure Science and Technology
Abstract

Investigação


Electronic states of heavy-fermion compounds under pressure combined with high magnetic field

Authors:
Yusuke Hirose (NU - Niigata University)

Abstract:

In rare earth and actinide compounds, fascinating electronic ground states such as magnetic ordering, heavy fermion, and unconventional superconductivity are realized as a result of RKKY interaction, Kondo effect, c-f hybridization. The electronic states in f-electron compounds can be tuned by pressure. For example, in some Ce compounds, the magnetic ordering temperature Tord decreases with increasing pressure and becomes zero at a critical pressure Pc, where a heavy fermion state and, sometimes, pressure-induced unconventional superconductivity are formed. In addition to pressure, the magnetic field is also important tool to investigate the electronic state of heavy-fermion compounds. In the high magnetic fields, for example, the tetragonal symmetry breaking and Fermi surface reconstruction in CeRhIn5 and field induced quadrupolar ordered phase in YbCo2Zn20 are observed[1-3].

In my talk, I focus on electronic states of some Ce based compounds under pressure and characteristic phase diagram of heavy-fermion compound CePt2In7 under pressure combined with pulsed-high-field using a new generation of pressure cells[4,5]. CePt2In7 exhibits an antiferromagnetic transition (AFM) at TN = 5.5 K [6]. TN is suppressed by the magnetic field and is expected to become zero at μ0Hc ~ 40 T for H || c axis [7,8]. TN is also suppressed by pressure above 2 GPa, and seems to become zero at PC ~ 3.2 GPa, where CePt2In7 shows the superconductivity (SC) with the highest transition temperature TSC ~ 2.1 K [9]. At 2.60 GPa, where AFM and SC coexist, AFM remains robust against the magnetic field and the SC critical field HC2 is expected to be higher than 10 T. However, restricted magnetic field and pressure windows have prevented from constructing the full (H,P,T) phase diagram.

From measurements of magnetization and magnetoresistance, the H-T phase diagrams of CePt2In7 for H || a and c axes are constructed as shown in figure, which is characterized by four states; paramagnetic (PM), correlated paramagnetic (CPM), antiferromagnetic (AF), and polarized paramagnetic (PPM) states. I show the pressure effects on phase diagram and relation between four states.

Figure: Phase diagram of CePt2In7 at ambient pressure.

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[2] F. Ronning, et al., Nature 548, 313 (2017).

[3] T. Takeuchi et al., J. Phys. Soc. Jpn. 80, 114703 (2011).

[4] R. Settai et al., Rev. High Press. Sci. and Tec 25, 325 (2015).

[5] D. Braithwaite et al., Rev. Sci. Instrum. 87, 023907 (2016).

[6] E. D. Bauer et al., Phys. Rev. B 81, 180507 (2010).

[7] M. M. Altarawneh et al., Phys. Rev. B 83, 081103 (2011).

[8] Y. Krupko et al., Phys. Rev. B 93, 085121 (2016).

[9] V. A. Sidorov et al., Phys. Rev. B 88, 020503 (2013).